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- W3201636893 abstract "Heterojunction construction has been proved to be an effective way to enhance photocatalysis performance. In this work, Cl-doped carbon nitride nanofibers (Cl-CNF) with broadband light harvesting capacity were in situ grown on carbon nitride nanosheets (CNS) by a facile hydrothermal method to construct a type II heterojunction. Benefiting from the joint effect of the improved charge carriers separation efficiency and a broadened visible light absorption range, the optimal heterostructure of Cl-CNF/CNS exhibits a H2O2 evolution rate of 247.5 μmol g-1 h-1 under visible light irradiation, which is 3.4 and 3.1 times as much as those of Cl-CNF (72.2 μmol g-1 h-1) and CNS (80.2 μmol g-1 h-1), respectively. Particularly, the heterojunction nanostructure displays an apparent quantum efficiency of 23.67% at 420 nm. Photoluminescence spectra and photocurrent measurements both verified the enhanced charge carriers separation ability. Our work provides a green and environmentally friendly strategy for H2O2 production by elaborate nanostructure design." @default.
- W3201636893 created "2021-09-27" @default.
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- W3201636893 date "2021-01-01" @default.
- W3201636893 modified "2023-10-11" @default.
- W3201636893 title "Growth of narrow-bandgap Cl-doped carbon nitride nanofibers on carbon nitride nanosheets for high-efficiency photocatalytic H<sub>2</sub>O<sub>2</sub> generation" @default.
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- W3201636893 doi "https://doi.org/10.1039/d1ra05787a" @default.
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