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- W3201664900 abstract "Silicon nanowires (Si NWs) are a promising anode material for lithium-ion batteries (LIBs) due to their high specific capacity. Achieving adequate mass loadings for binder-free Si NWs is restricted by low surface area, mechanically unstable and poorly conductive current collectors (CCs), as well as complicated/expensive fabrication routes. Herein, a tunable mass loading and dense Si NW growth on a conductive, flexible, fire-resistant, and mechanically robust interwoven stainless-steel fiber cloth (SSFC) using a simple glassware setup is reported. The SSFC CC facilitates dense growth of Si NWs where its open structure allows a buffer space for expansion/contraction during Li-cycling. The Si NWs@SSFC anode displays a stable performance for 500 cycles with an average Coulombic efficiency of >99.5%. Galvanostatic cycling of the Si NWs@SSFC anode with a mass loading of 1.32 mg cm-2 achieves a stable areal capacity of ≈2 mAh cm-2 at 0.2 C after 200 cycles. Si NWs@SSFC anodes with different mass loadings are characterized before and after cycling by scanning and transmission electron microscopy to examine the effects of Li-cycling on the morphology. Notably, this approach allows the large-scale fabrication of robust and flexible binder-free Si NWs@SSFC architectures, making it viable for practical applications in high energy density LIBs." @default.
- W3201664900 created "2021-10-11" @default.
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- W3201664900 date "2021-10-22" @default.
- W3201664900 modified "2023-10-10" @default.
- W3201664900 title "Dense Silicon Nanowire Networks Grown on a Stainless‐Steel Fiber Cloth: A Flexible and Robust Anode for Lithium‐Ion Batteries" @default.
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- W3201664900 doi "https://doi.org/10.1002/adma.202105917" @default.
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