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• W3201722146 abstract "Polymer nanocapsules have demonstrated significant value in materials science and biomedical technology, but require complicated and time-consuming synthetic steps. We report here the facile synthesis of monodisperse polymer nanocapsules via a redox-mediated kinetic strategy from two simple molecules: dopamine and benzene-1,4-dithiol (BDT). Specifically, BDT forms core templates and modulates the oxidation kinetics of dopamine into polydopamine (PDA) shells. These uniform nanoparticles can be tuned between ≈70 and 200 nm because the core diameter directly depends on BDT while the shell thickness depends on dopamine. The supramolecular core can then rapidly disassemble in organic solvents to produce PDA nanocapsules. Such nanocapsules exhibit enhanced physicochemical performance (e.g., loading capacity, photothermal transduction, and anti-oxidation) versus their solid counterparts. Particularly, this method enables a straightforward encapsulation of functional nanoparticles providing opportunities for designing complex nanostructures such as yolk-shell nanoparticles." @default.
• W3201722146 created "2021-10-11" @default.
• W3201722146 creator A5002893358 @default.
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• W3201722146 date "2021-11-05" @default.
• W3201722146 modified "2023-10-18" @default.
• W3201722146 title "Versatile Polymer Nanocapsules via Redox Competition" @default.
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• W3201722146 doi "https://doi.org/10.1002/anie.202110829" @default.
• W3201722146 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/8629958" @default.
• W3201722146 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34580967" @default.
• W3201722146 hasPublicationYear "2021" @default.
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