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- W3201753419 abstract "The persistent problem posed by the glass transition is to develop a general atomic level description of a solidification process that is not associated with any change in the symmetry of the atomic structure. The answer proposed in this paper is to measure a configuration's capacity to restrain the motion of the constituent atoms. Previous efforts based on local topologies run up against the sheer diversity of disordered structures. Unlike crystals, an amorphous solid can have more than 100 local topological arrangements. The random first order transition theory enlists a related overlap parameter but this characterizes a metastable state, not the mechanical restraint of a single configuration that we need. Here we show that the instantaneous normal modes can be used to define a transparent measure of atomic restraint that accounts for the difference between fragile and strong liquids and the collective length scale of the supercooled liquid. We show that amorphous solidifcation proceeds unchanged when we exclude the selection of favoured local structures and cooperative phase behaviour through ultra-rapid cooling. These results represents a significant simplification of the description of amorphous solidification and a powerful systematic treatment of the influence of microscopic factors based on the structural description presented here." @default.
- W3201753419 created "2021-10-11" @default.
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- W3201753419 date "2021-09-26" @default.
- W3201753419 modified "2023-09-27" @default.
- W3201753419 title "The Structural Transformation of a Supercooled Liquid into an Amorphous Solid" @default.
- W3201753419 hasPublicationYear "2021" @default.
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