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• W3201866897 endingPage "2104623" @default.
• W3201866897 startingPage "2104623" @default.
• W3201866897 abstract "Protonated 3d transition-metal oxides often display low electronic conduction, which hampers their application in electric, magnetic, thermoelectric, and catalytic fields. Electronic conduction can be enhanced by co-inserting oxygen acceptors simultaneously. However, the currently used redox approaches hinder protons and oxygen ions co-insertion due to the selective switching issues. Here, a thermal hydration strategy for systematically exploring the synthesis of conductive protonated oxides from 3d transition-metal oxides is introduced. This strategy is illustrated by synthesizing a novel layered-oxide SrCoO3H from the brownmillerite SrCoO2.5. Compared to the insulating SrCoO2.5, SrCoO3H exhibits an unprecedented high electronic conductivity above room temperature, water uptake at 250 °C, and a thermoelectric power factor of up to 1.2 mW K−2 m−1 at 300 K. These findings open up opportunities for creating high-conductive protonated layered oxides by protons and oxygen ions co-doping." @default.
• W3201866897 created "2021-10-11" @default.
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• W3201866897 date "2021-09-29" @default.
• W3201866897 modified "2023-10-11" @default.
• W3201866897 title "High‐Conductive Protonated Layered Oxides from H ₂ O Vapor‐Annealed Brownmillerites" @default.
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• W3201866897 doi "https://doi.org/10.1002/adma.202104623" @default.
• W3201866897 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34590356" @default.
• W3201866897 hasPublicationYear "2021" @default.
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