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• W3201916462 abstract "Studies of Ni–yttria-stabilized zirconia (YSZ) fuel electrode degradation mechanisms in solid oxide electrolysis cells (SOECs) are complicated by the different possible Ni–YSZ microstructures and compositions, and the variations in the H2/H2O ratio encountered in an electrolysis stack. Here we describe a life testing scheme aimed at providing survey results on degradation as a function of the H2O–H2 composition, with life tests carried out at five different steam contents from 90% to 10%. A Ni–YSZ-supported symmetric cell geometry is employed both with and without infiltrated nanoscale gadolinia-doped ceria (GDC). Impedance spectroscopy is utilized to observe changes in electrochemical characteristics during the life test, and a transmission-line-based equivalent circuit is used to model the data. Post-test electrode microstructures were observed. The results suggest that the GDC infiltrant reduces the electrode polarization resistance and provides more stable electrode polarization over a range of conditions." @default.
• W3201916462 created "2021-10-11" @default.
• W3201916462 creator A5008017115 @default.
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• W3201916462 date "2021-10-04" @default.
• W3201916462 modified "2023-10-16" @default.
• W3201916462 title "Effect of Nanoscale Ce_0.8Gd_0.2O_2−δ Infiltrant and Steam Content on Ni–(Y₂O₃)_0.08(ZrO₂)_0.92 Fuel Electrode Degradation during High-Temperature Electrolysis" @default.
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• W3201916462 doi "https://doi.org/10.1021/acs.nanolett.1c02937" @default.
• W3201916462 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34606281" @default.
• W3201916462 hasPublicationYear "2021" @default.
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