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• W3202021644 abstract "High-performance hole-transporting materials (HTMs) play an essential role in improving efficiency and stability of perovskite solar cells (PSCs). Herein, we developed a new sulfonyldibenzene core based HTM named CS-06 , which contains substituted fluorene-terminated moieties as end groups in molecular structure. It is found that, the substituted fluorene-terminated end groups render CS-06 with a deep HOMO level, high hole mobility and glass transition temperature, which are beneficial for improving hole extraction and decreasing recombination probabilities at HTM/perovskite interface. The champion device based on CS-06 can yield a power conversion efficiency of 21.10%, superior to devices based on its analog CS-04 (19.73%) as reference. This work provides an effective way to develop efficient HTMs through rational end group design to boost the photovoltaic performance of PSCs. • A sulfonyldibenzene-core based hole-transporting material ( CS-06 ) by end group engineering. • CS-06 exhibits high hole mobility, suitable energy level and good film quality. • CS-06 enabled perovskite solar cells with high efficiency (PCE = 21.10%) and stability." @default.
• W3202021644 created "2021-10-11" @default.
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• W3202021644 date "2022-01-01" @default.
• W3202021644 modified "2023-10-17" @default.
• W3202021644 title "A hole-transporting material with substituted fluorene as end groups for high-performance perovskite solar cells" @default.
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• W3202021644 doi "https://doi.org/10.1016/j.orgel.2021.106325" @default.
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