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- W3202068248 abstract "Water splitting will become important to store excess renewable electrical energy into hydrogen. Although the oxygen-evolution reaction (OER) by water oxidation is a critical reaction for water splitting, further investigations are needed to find the details of the OER mechanism for various electrocatalysts. More in particular for homogeneous electrocatalysts, the Randles-Sevcik equation has been extensively applied to determine the turnover frequency (TOF). Herein, using vitamin B12 as a case study, we show that the dynamical deposition/dissolution of the heterogeneous catalyst during OER makes the Randles-Sevcik equation too complicated to be used for calculating the TOF. Indeed, the conventionally applied post-characterization methods do not provide sufficient accuracy to prove the homogeneity of OER mechanisms; thus, using the Randles-Sevcik equation to calculate the TOF is not necessarily correct." @default.
- W3202068248 created "2021-10-11" @default.
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- W3202068248 date "2021-11-01" @default.
- W3202068248 modified "2023-10-10" @default.
- W3202068248 title "The importance of identifying the true catalyst when using Randles-Sevcik equation to calculate turnover frequency" @default.
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- W3202068248 doi "https://doi.org/10.1016/j.ijhydene.2021.09.039" @default.
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