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- W3202107457 abstract "Due to the high theoretical specific capacity and low cost, FeF3·0.33H2O has become one of the potential choices of cathode materials for sodium-ion batteries. However, the poor intrinsic conductivity limits its practical applications. Herein, the atomic substitution is used to improve its intrinsic conductivity. The first-principles calculation results show that Cr3+ doping can reduce the band gap of FeF3·0.33H2O to improve its intrinsic conductivity. The discharge specific capacity of Fe0.95Cr0.05F3·0.33H2O with a narrowest band gap is 194.02 mA h/g at 0.1 C within the range of 1.4-4.0 V, which is higher than that of FeF3·0.33H2O (136.47 mA h/g). Using the electrochemical impedance spectroscopy and galvanostatic intermittent titration technique tests, it is found that Rct of Fe0.95Cr0.05F3·0.33H2O is reduced and DNa+ is almost unchanged, as compared to FeF3·0.33H2O." @default.
- W3202107457 created "2021-10-11" @default.
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- W3202107457 date "2021-10-06" @default.
- W3202107457 modified "2023-09-23" @default.
- W3202107457 title "Cr-Doped Fe1–xCrxF3·0.33H2O Nanomaterials as Cathode Materials for Sodium-Ion Batteries" @default.
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- W3202107457 doi "https://doi.org/10.1021/acsami.1c13462" @default.
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