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- W3202393231 endingPage "48817" @default.
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- W3202393231 abstract "Low-temperature operation is a challenge for solid-lithium-metal batteries (LMBs), and insufficient ionic conductivity is the main obstacle. Herein, guided by the molecular dynamics simulations (MDS), a solid polymer electrolyte (SPE) based on poly(1,3-dioxolane) (PDOL) with sufficient ionic conductivity at low temperature is reported. In situ X-ray diffraction (XRD) and differential scanning calorimetry (DSC) tests reveal that the PDOL-based SPE could well maintain amorphous nature at low temperatures, contributing to excellent ionic transport. The MDS analysis of the Li-O coordination environment indicates that more oxygen atoms bonded with Li+ in PDOL than in poly(ethylene oxide) (PEO) at low temperatures, thus we could envision the preponderance of PDOL as a better polymer matrix of SPE for low-temperature solid LMBs. It delivers a high capacity of 103 mAh g-1 and 85% retention for 200 cycles for Li||LiFePO4 at -20 °C, showing great potential for application in low-temperature solid LMBs in cold climates." @default.
- W3202393231 created "2021-10-11" @default.
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- W3202393231 date "2021-10-07" @default.
- W3202393231 modified "2023-10-17" @default.
- W3202393231 title "Molecular Simulations Guided Polymer Electrolyte towards Superior Low-Temperature Solid Lithium-Metal Batteries" @default.
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- W3202393231 doi "https://doi.org/10.1021/acsami.1c14825" @default.
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