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• W3203084687 endingPage "139106" @default.
• W3203084687 startingPage "139106" @default.
• W3203084687 abstract "• Normal Raman spectra suggests only dispersion forces between ions and SO 2 . • Resonance Raman spectra evidences charge transfer interactions between TCM and SO 2 . • The charge transfer solvation states contribute to the high absorption of SO 2 . Interactions concerning the high SO 2 absorption capacity in 1-butyl-3-methyilimidazolium tricyanomethanide (BMITCM) were analyzed through Raman spectroscopy. The SO 2 symmetric stretching band, ν s (SO 2 ), remained equal in shape and wavenumber regardless the SO 2 molar fraction, suggesting no specific interaction between TCM and SO 2 . However, by increasing the Raman excitation energy from 568 to 405 nm, a pre-resonance condition was reached, where a shifting and broadening of ν s (SO 2 ) is noticed. Such results evidence solvation states where charge transfer interactions between TCM and SO 2 prevail, corroborating the high absorption capacity of TCM based ionic liquids." @default.
• W3203084687 created "2021-10-11" @default.
• W3203084687 creator A5003090183 @default.
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• W3203084687 date "2021-12-01" @default.
• W3203084687 modified "2023-10-12" @default.
• W3203084687 title "SO2 capture by tricyanomethanide ionic liquids: Unraveling anion-gas interactions by resonance Raman spectroscopy" @default.
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• W3203084687 doi "https://doi.org/10.1016/j.cplett.2021.139106" @default.
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