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• W3203205495 endingPage "139090" @default.
• W3203205495 startingPage "139090" @default.
• W3203205495 abstract "• Using the real-space implemented self-consistent field theory, the concentric structure-in-structure (B- enwrap -C) and surface-patched structure-on-structure (B- patch -C) multicompartment micelles were observed by tailoring the B block lengths. • It was found that the formation of B- patch -C is driven by the conformational entropy of the B blocks. • An unusual morphological evolution from raspberry-like to concentric multicompartment micelles was discovered and proven to be driven by the conformational entropy of the inner blocks of the A- g -BC graft terpolymer backbone. The self-assembly behaviors and morphological evolutions of the A- g -BC graft terpolymers in A-backbone-attractive solvents were examined by using the real-space implemented self-consistent field theory. The concentric structure-in-structure (B- enwrap -C) and surface-patched structure-on-structure (B- patch -C) multicompartment micelles were observed by tailoring the B block lengths. At longer length of B blocks, the A- g -BC graft terpolymers prefer to form the common concentric B- enwrap -C multicompartment micelles, while the B- patch -C multicompartment micelles with B patches on C surface favor the shorter length of B blocks. It was found that the formation of B- patch -C is driven by the conformational entropy of the B blocks. In addition, when the length of B block decreases into a much lower value, an unusual morphological evolution from raspberry-like to concentric multicompartment micelles was discovered, which was revealed to be driven by the conformational entropy of the inner blocks of A backbone between two adjacent graft points. The gained results could provide a deep insight into the mechanism behind the morphological evolution between concentric structure-in-structure (B- enwrap -C) and surface-patched structure-on-structure (B- patch -C) multicompartment micelles." @default.
• W3203205495 created "2021-10-11" @default.
• W3203205495 creator A5073568638 @default.
• W3203205495 creator A5083885063 @default.
• W3203205495 date "2021-12-01" @default.
• W3203205495 modified "2023-09-23" @default.
• W3203205495 title "Discovery of unusual morphological evolution of A-graft-(B-block-C) graft terpolymers by tuning the length of B component" @default.
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• W3203205495 doi "https://doi.org/10.1016/j.cplett.2021.139090" @default.
• W3203205495 hasPublicationYear "2021" @default.
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