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• W3203206211 abstract "Using a newly developed two-step hydrothermal process, flowerlike Ce 0.5 Zr 0.5 O 2 with an oxygen storage capacity (OSC) of 536 μmol O 2 g −1 , almost twice as high as that of pure flowerlike CeO 2 (284 μmol O 2 g −1 ), can be synthesized. The synthesized ceria-based oxide supports loaded with Ni are dispersed in a ceramic fiber network to form paper-structured catalysts (PSCs). Among the prepared PSCs, the PSC with the flowerlike Ce 0.5 Zr 0.5 O 2 exhibits the highest catalytic performance for dry reforming of methane (DRM) at 750 °C with the initial methane conversion of 88.4%, degradation rate of 0.1% h −1 and amount of deposited carbon of 0.04 g per gram catalyst, whereas for the Ce 0.5 Zr 0.5 O 2 synthesized by the one-step hydrothermal process, the values are 83.7%, 0.62% h −1 and 0.07 g per gram catalyst, respectively. This is attributed to the Ni anti-sintering on the petals of the flowerlike structure and the coking tolerance resulting from the high OSC. • Flowerlike Ce 0.5 Zr 0.5 O 2 could be synthesized by a two-step hydrothermal process. • OSC of the flowerlike Ce 0.5 Zr 0.5 O 2 , 536 μmol O 2 g −1 , was twice as high as pure CeO 2 . • Ceria-based oxides with Ni were dispersed in a ceramic fiber network to form PSCs. • PSC with flowerlike Ni/Ce 0.5 Zr 0.5 O 2 showed the highest catalytic performance for DRM. • Both high OSC and flowerlike geometry of the Ce 0.5 Zr 0.5 O 2 contributed to anti-coking." @default.
• W3203206211 created "2021-10-11" @default.
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• W3203206211 date "2022-12-01" @default.
• W3203206211 modified "2023-09-23" @default.
• W3203206211 title "Synthesis of flowerlike ceria–zirconia solid solution for promoting dry reforming of methane" @default.
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• W3203206211 doi "https://doi.org/10.1016/j.ijhydene.2021.09.025" @default.
• W3203206211 hasPublicationYear "2022" @default.
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