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- W3203490457 abstract "The diversity and wide availability of trialkylamines render them ideal sources for rapid construction of complex amine architectures. Herein, we report that a nickel/photoredox dual catalysis strategy affects site-selective α-arylation of various trialkylamines. Our catalytic system shows exclusive N-Me selectivity with a wide range of trialkylamines under mild conditions, even in the context of late-stage arylation of pharmaceutical compounds bearing this common structural motif. Mechanistic studies indicate the unconventional behavior of Ni catalyst upon intercepting the α-amino radicals, in which only the primary α-amino radical undergoes a successful cross-coupling process." @default.
- W3203490457 created "2021-10-11" @default.
- W3203490457 creator A5069701929 @default.
- W3203490457 creator A5074994681 @default.
- W3203490457 date "2021-09-30" @default.
- W3203490457 modified "2023-10-03" @default.
- W3203490457 title "Late-Stage <i>N</i>-Me Selective Arylation of Trialkylamines Enabled by Ni/Photoredox Dual Catalysis" @default.
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- W3203490457 doi "https://doi.org/10.1021/jacs.1c08157" @default.
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- W3203490457 hasPublicationYear "2021" @default.
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