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- W3203993333 abstract "Abstract A series of poly(phenylene-vinylene)-based copolymers are synthesized using the Gilch method incorporating monomers with sterically bulky sidechains. The photochemical upconversion performance of these polymers as emitters are investigated using a palladium tetraphenyltetrabenzoporphyrin triplet sensitizer and MEH-PPV as reference. Increased incorporation of sterically bulky monomers leads to a reduction in the upconversion efficiency despite improved photoluminescence quantum yield. A phosphorescence quenching study indicates issues with the energy transfer process between the triplet sensitizer and the copolymers. The best performance with 0.18% upconversion quantum yield is obtained for the copolymer containing 10% monomer with bulky sidechains." @default.
- W3203993333 created "2021-10-11" @default.
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- W3203993333 date "2021-10-01" @default.
- W3203993333 modified "2023-10-14" @default.
- W3203993333 title "Revealing the influence of steric bulk on the triplet–triplet annihilation upconversion performance of conjugated polymers" @default.
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- W3203993333 doi "https://doi.org/10.1038/s41598-021-99179-y" @default.
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