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- W3204057218 endingPage "117160" @default.
- W3204057218 startingPage "117160" @default.
- W3204057218 abstract "It is significantly valuable to convert p-nitrophenol to p-aminophenol by catalysis. Herein, a novel [email protected]/CM catalytic membrane was synthesized, where ZIF-67 was first in-situ grown on the surface and in the pores of a ceramic membrane (CM) and then pyrolyzed to produce [email protected] carbon ([email protected]). The calcination temperature and Co2+ concentration significantly affect the microstructure of [email protected]/CM-X-Y (X represents the Co2+ molar concentration in methanol solution and Y represents the calcination temperature), and the corresponding catalytic properties for the p-nitrophenol reduction. The as-fabricated catalytic membrane [email protected]/CM-0.6–900 exhibits a superior catalytic activity, with a p-nitrophenol conversion of above 99% within 10 min, which is three times higher than that of [email protected]/CM-0.6–400. [email protected]/CM-0.6–900 also shows excellent reusability during five hydrogenation cycles. Abundant mesopores, high flux, many relatively isolated [email protected] particles with higher Co0 content, high N-pyrrolic content, and the protection function of CN are the reasons for the superior catalytic performance of [email protected]/CM-0.6–900." @default.
- W3204057218 created "2021-10-11" @default.
- W3204057218 creator A5013913370 @default.
- W3204057218 creator A5067937296 @default.
- W3204057218 creator A5074997400 @default.
- W3204057218 date "2022-02-01" @default.
- W3204057218 modified "2023-10-15" @default.
- W3204057218 title "Synthesis of ZIF-67 derived Co-based catalytic membrane for highly efficient reduction of p-nitrophenol" @default.
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- W3204057218 doi "https://doi.org/10.1016/j.ces.2021.117160" @default.
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