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- W3204132852 abstract "Metallo-polyelectrolytes have been demonstrated to be promising candidates for anion exchange membranes (AEMs) due to their excellent alkaline stability. Here, cobaltocenium-containing metallo-polyelectrolyte-based AEMs with good chemical stability and dimensional stability were prepared through facile acetalation of a commodity polymer, poly(vinyl alcohol). The AEM crosslinked with 1 wt % glutaraldehyde (GA) exhibits a comparable hydroxide conductivity of 72 mS/cm at 80 °C and enhanced alkaline stability in 1 M NaOH at 80 °C (maintained 86.3% of initial hydroxide conductivity after 1000 h). The dimensional stability of these AEMs can be tuned through acetalation crosslinking with GA, and the swelling ratio of 1% GA was 17.8% and the gel fraction was 90.5%. The H2/O2 single cell using 1% GA AEM (50 μm, Fumion ionomer) showed a maximum power density of 120 mW/cm2 at 60 °C without backpressure. This work provides a facile method for the preparation of stable metallo-polyelectrolyte-based alkaline membrane fuel cells." @default.
- W3204132852 created "2021-10-11" @default.
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- W3204132852 date "2021-09-29" @default.
- W3204132852 modified "2023-10-16" @default.
- W3204132852 title "Metallo-Polyelectrolyte-Based Robust Anion Exchange Membranes via Acetalation of a Commodity Polymer" @default.
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- W3204132852 doi "https://doi.org/10.1021/acs.macromol.1c01346" @default.
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