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• W3204137899 abstract "Abstract We explore crystallisation and polymorph selection in active Brownian particles with numerical simulation. In agreement with previous work (Wysocki et al. in Europhys Lett 105:48004, 2014), we find that crystallisation is suppressed by activity and occurs at higher densities with increasing Péclet number ( $${ Pe }$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mrow> <mml:mi>Pe</mml:mi> </mml:mrow> </mml:math> ). While the nucleation rate decreases with increasing activity, the crystal growth rate increases due to the accelerated dynamics in the melt. As a result of this competition, we observe the transition from a nucleation and growth regime at high $${ Pe }$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mrow> <mml:mi>Pe</mml:mi> </mml:mrow> </mml:math> to “spinodal nucleation” at low $${ Pe }$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mrow> <mml:mi>Pe</mml:mi> </mml:mrow> </mml:math> . Unlike the case of passive hard spheres, where preference for FCC over HCP polymorphs is weak, activity causes the annealing of HCP stacking faults, thus strongly favouring the FCC symmetry at high $${ Pe }$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mrow> <mml:mi>Pe</mml:mi> </mml:mrow> </mml:math> . When freezing occurs more slowly, in the nucleation and growth regime, this tendency is much reduced and we see a trend towards the passive case of little preference for either polymorph." @default.
• W3204137899 created "2021-10-11" @default.
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• W3204137899 date "2021-09-01" @default.
• W3204137899 modified "2023-10-17" @default.
• W3204137899 title "Crystallisation and polymorph selection in active Brownian particles" @default.
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• W3204137899 doi "https://doi.org/10.1140/epje/s10189-021-00108-8" @default.
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