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• W3204156997 abstract "The state-of-the-art solar-thermal evaporators demonstrating high energy utilization efficiency, a high evaporation rate, and salt rejection are highly desirable in solar-driven low-energy water purification/harvesting. Herein, a novel Janus solar evaporator is constructed by loading polypyrrole (PPy) nanobelts on the polyvinyl alcohol (PVA) hydrogel. The PPy nanobelts present a high solar absorption of 98.3%, leading to a localized solar-thermal efficiency of 82.5% when insulated from bulk water by the PVA hydrogel. The porous PVA hydrogel and the hydrophilic PPy nanobelts enable the efficient three-dimensional water transport. Taking advantages of the synergistic effect in the water-energy nexus, the Janus PPy nanobelt@PVA hydrogel evaporator evaporates water with a high rate of 2.26 kg m–2 h–1 via 80.1% solar energy from 1 sun irradiance with a low PPy loading of ∼3 mg cm–2 even at a rate of 2.64 kg m–2 h–1 via 96.3% solar energy for a biomimetic conical evaporator. The Janus evaporator presents superior salt-resistant desalination and contaminant purification performance in seawater and sewage. Furthermore, a portable solar-thermal purifier equipped with the Janus evaporator desalts real seawater far above the drinking water standard with over a 99.9% salt rejection rate and eliminates 95.8% of chemical oxygen demand in real sewage, highlighting its potential for advanced clean water harvesting." @default.
• W3204156997 created "2021-10-11" @default.
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• W3204156997 date "2021-09-27" @default.
• W3204156997 modified "2023-10-16" @default.
• W3204156997 title "Janus Polypyrrole Nanobelt@Polyvinyl Alcohol Hydrogel Evaporator for Robust Solar-Thermal Seawater Desalination and Sewage Purification" @default.
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• W3204156997 doi "https://doi.org/10.1021/acsami.1c13584" @default.
• W3204156997 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34569244" @default.
• W3204156997 hasPublicationYear "2021" @default.
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