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• W3204244242 abstract "Non-phase-separated hexagonal boron carbon nitride (h-BCN) is an emerging type of promising metal-free photocatalyst, but the synthesis of this material remains quite challenging. Here, h-BCN without phase separation was obtained through a novel organic-inorganic hybrid precursor pyrolysis method using boric acid and ethylenediamine as raw materials. The resultant BCN-1 exhibited excellent photocatalytic activity for CO2 reduction, as confirmed by a CO generation rate of 13.97 μmol g-1 h-1 under visible light illumination with no co-catalyst or sacrificial agent. This rate was 9.4 times higher than that of g-C3N4 (2.1 μmol g-1 h-1) under the same experimental condition. The pre-existing C-N-B bond is essential for mediating the growth kinetics and diminishing the thermodynamically preferred C and BN phase-segregation structure, while ammonia is crucial for C-N-B bond fixation and pore formation during the pyrolysis process. This finding of a facile method for synthesizing non-phase-separated BCN has positive effects on the study of photocatalytic CO2 reduction by sustainable metal-free catalysts." @default.
• W3204244242 created "2021-10-11" @default.
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• W3204244242 date "2022-05-01" @default.
• W3204244242 modified "2023-10-14" @default.
• W3204244242 title "In-situ synthesis of non-phase-separated boron carbon nitride for photocatalytic reduction of CO2" @default.
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• W3204244242 doi "https://doi.org/10.1016/j.envres.2021.112178" @default.
• W3204244242 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34624270" @default.
• W3204244242 hasPublicationYear "2022" @default.
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