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• W3204268656 abstract "Reversible solid oxide cell (RSOC) technology allows use of a single device to efficiently derive chemicals from power (power-to-fuel) and power from chemicals (fuel-to-power). Fuel flexibility is a key aspect, as developing SOCs able to operate on fuels other than hydrogen can ease their integration into existing infrastructure. In addition, H2O and/or CO2 reduction is favorable in SOECs as polarization losses are reduced at high temperature. Here, a composite fuel electrode, 60 wt.% La0.6Sr0.4Fe0.8Mn0.2O3−δ (LSFMn) and 40 wt.% (5 wt.% Ni)-containing Ce0.85Sm0.15O2−δ (Ni-SDC) was investigated in H2-fueled, CO-fueled SOFCs and for CO2 reduction in SOEC mode. In reducing conditions, Fe exsolved from the LSFMn perovskite formed a Ni–Fe alloy with Ni present on SDC. The composite fuel electrode showed remarkable activity for CO2 reduction with a current density output of 1.40 A cm−2 (1.5 V) at 850 °C. SOFC/SOEC cell reversibility was obtained in different CO2:CO mixtures. Electrochemical impedance spectroscopy analysis was used to better understand cell mechanisms in SOFC and SOEC mode." @default.
• W3204268656 created "2021-10-11" @default.
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• W3204268656 date "2021-10-01" @default.
• W3204268656 modified "2023-09-26" @default.
• W3204268656 title "Novel Composite Fuel Electrode for CO₂/CO-RSOCs" @default.
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• W3204268656 doi "https://doi.org/10.1149/1945-7111/ac2c15" @default.
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