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- W3204285738 endingPage "127387" @default.
- W3204285738 startingPage "127387" @default.
- W3204285738 abstract "In the conventional Fenton system, the relatively low efficiency of Fe (II) regeneration is a significant drawback. To address this shortcoming, a novel floating Z-scheme photo-Fenton catalyst FeMo3Ox/g-C3N4/EP was prepared by a facile dip-calcination method, in which iron and molybdenum oxides with mixed valence states (FeMo3Ox) and graphitic carbon nitride (g-C3N4) were loaded on the expanded perlite. The removal efficiencies reached the maximum at 98.0%, 93.1% and 97.1% for tetracycline, oxytetracycline and chlortetracycline, respectively, after 60 min dark adsorption and 60 min photo-Fenton process. The aid of dual ion (Fe and Mo) synergy system and photoreduction by Z-scheme photocatalyst enhanced the Fe (II) regeneration, resulting in the excellent performance. Radical scavenger experiment, electron spin resonance spectra (ESR) and X-ray photoelectron spectra (XPS) were used to confirm the mechanism of free radicals' formation and Fe/Mo redox cycling. ·OH, ·O2- and 1O2 played important roles in the pollutant's degradation, while the generation of ·O2- was enhanced due to the floatability in this system. The possible degradation pathways of TC were put forward according to the results of mass spectrum and Orbital-Weighted Fukui Function. Overall, this work provides new insights on the cooperation between iron-based mix oxides and semiconductor in the photo-Fenton system." @default.
- W3204285738 created "2021-10-11" @default.
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- W3204285738 date "2022-02-01" @default.
- W3204285738 modified "2023-10-16" @default.
- W3204285738 title "Enhanced visible light photo-Fenton-like degradation of tetracyclines by expanded perlite supported FeMo3Ox/g-C3N4 floating Z-scheme catalyst" @default.
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- W3204285738 doi "https://doi.org/10.1016/j.jhazmat.2021.127387" @default.
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- W3204285738 hasPublicationYear "2022" @default.
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