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• W3204407337 abstract "The high interfacial resistance between solid electrolytes and lithium metal is a hurdle to developing all solid-state batteries. External pressure applied on the lithium and solid electrolyte interface prior to electrochemical cycling is known to effectively lower the interfacial resistance. Here we report that the interfacial resistance between Li6.4La3Zr1.4Ta0.6O12 (LLZTO) and lithium metal decreases over time even after removing the external pressure. The irreversible decrease of interfacial resistance can be understood by a gradual reduction of the total energy of the system, including strain energy and interfacial energy. Under external pressure exceeding ∼25 MPa, however, lithium can be squeezed into LLZTO, fracturing the ceramic solid electrolyte. These observations can help improve the understanding of lithium metal creep and the interactions between garnet-type solid electrolytes and lithium metal." @default.
• W3204407337 created "2021-10-11" @default.
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• W3204407337 date "2021-10-01" @default.
• W3204407337 modified "2023-09-23" @default.
• W3204407337 title "A Power-Law Decrease in Interfacial Resistance Between Li₇La₃Zr₂O₁₂ and Lithium Metal After Removing Stack Pressure" @default.
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• W3204407337 doi "https://doi.org/10.1149/1945-7111/ac2d43" @default.
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