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- W3204459570 abstract "A palladium-catalyzed enantioselective Heck cyclization/dearomatization cascade via capturing the cyclized Heck π-allylpalladium intermediate by β-naphthols is reported, which provides a new strategy for the construction of chiral indole-terpenoid frameworks. This method affords indole-functionalized β-naphthalenone compounds bearing an all-carbon-substituted quaternary chiral center in excellent yields (up to 92%) and enantioselectivities (up to 94% ee). In addition, the utility of this method is showcased by the gram-scale syntheses and diverse transformations of the dearomatized products." @default.
- W3204459570 created "2021-10-11" @default.
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- W3204459570 date "2021-09-28" @default.
- W3204459570 modified "2023-10-10" @default.
- W3204459570 title "Asymmetric Domino Heck/Dearomatization Reaction of β-Naphthols to Construct Indole–Terpenoid Frameworks" @default.
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- W3204459570 doi "https://doi.org/10.1021/acs.orglett.1c02881" @default.
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