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- W3204662194 abstract "The assembly of two tripyridinium-tricarboxylate ligands and different metal ions leads to seven isostructural MOFs, which show novel 2D→2D supramolecular entanglement featuring catenane-like interlocking of tricyclic cages. The MOFs show tripyridinium-afforded and metal-modulated photoresponsive properties. The MOFs with d10 metal centers (1-Cd, 1-Zn, 2-Cd, 2-Zn) show fast and reversible photochromism and concomitant fluorescence quenching, 1-Ni displays slower photochromism but does not fluoresce, and 1-Co and 2-Co are neither photochromic nor fluorescent. It is shown here that the network entanglement dictates donor-acceptor close contacts, which enable fluorescence originated from interligand charge transfer. The contacts also allow photoinduced electron transfer, which underlies photochromism and concomitant fluorescence response. The metal dependence in fluorescence and photochromism can be related to energy transfer through metal-centered d-d transitions. In addition, 1-Cd is demonstrated to be a potential fluorescence sensor for sensitive and selective detection of UO22+ in water." @default.
- W3204662194 created "2021-10-11" @default.
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- W3204662194 date "2021-10-21" @default.
- W3204662194 modified "2023-10-17" @default.
- W3204662194 title "Metal‐Organic Frameworks with Novel Catenane‐like Interlocking: Metal‐Determined Photoresponse and Uranyl Sensing" @default.
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- W3204662194 doi "https://doi.org/10.1002/chem.202102413" @default.
- W3204662194 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34599532" @default.
- W3204662194 hasPublicationYear "2021" @default.
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