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• W3204761122 endingPage "127315" @default.
• W3204761122 startingPage "127315" @default.
• W3204761122 abstract "The emerging contaminants polyhalogenated carbazoles (PHCZs) have been verified to be present in soils and sediments globally, and they show dioxin-like toxicity. However, there is a lack of soil ecological risk assessments on PHCZs despite their high detection rate and concentration in soils. The present study investigated the degradation and soil microbial influence of 3,6-dichlorocarbazole (3,6-DCCZ, a frequently detected PHCZ) in soil. The results showed that the half-lives of 3,6-DCCZ at concentrations of 0.100 mg/kg and 1.00 mg/kg were 7.75 d and 16.73 d, respectively. We found that 3,6-DCCZ was transformed into 3-chlorocarbazole (3-CCZ) by dehalogenation in soil. Additionally, intermediate products with higher molecular weights were detected, presumably because the -H on the carbazole ring was replaced by -CH3, -CH2-O-CH3, or -CH2-O-CH2CH3. 3,6-DCCZ exposure slightly increased the soil bacterial abundance and diversity and clearly changed the soil bacterial community structure. Through a comprehensive analysis of FAPROTAX, functional gene qPCR and soil enzyme tests, we concluded that 3,6-DCCZ exposure inhibited nitrification and nitrogen fixation but promoted denitrification, carbon dioxide fixation and hydrocarbon degradation processes in soil. This study provides valuable data for clarifying the PHCZ ecological risk in soil." @default.
• W3204761122 created "2021-10-11" @default.
• W3204761122 creator A5029457967 @default.
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• W3204761122 date "2022-02-01" @default.
• W3204761122 modified "2023-10-14" @default.
• W3204761122 title "Effects of 3,6-dichlorocarbazole on microbial ecology and its degradation in soil" @default.
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• W3204761122 doi "https://doi.org/10.1016/j.jhazmat.2021.127315" @default.
• W3204761122 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34601412" @default.
• W3204761122 hasPublicationYear "2022" @default.
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