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- W3204823545 abstract "Peptidoglycans are diverse co- and post-translational modifications of key importance in myriad biological processes. Mass spectrometry is employed to infer their biomolecular sequences and stereochemisties, but little is known about the critical gas-phase dissociation processes involved. Here, using tandem mass spectrometry (MS/MS and MSn), isotopic labelling and high-level simulations, we identify and characterize a facile isomerization reaction that produces furanose N-acetylated ions. This reaction occurs for both O- and N-linked peptidoglycans irrespective of glycosidic linkage stereochemistry (α/β). Dissociation of the glycosidic and other bonds thus occur from the furanose isomer critically altering the reaction feasibility and product ion structures." @default.
- W3204823545 created "2021-10-11" @default.
- W3204823545 creator A5021915667 @default.
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- W3204823545 date "2021-01-01" @default.
- W3204823545 modified "2023-10-10" @default.
- W3204823545 title "Evidence of gas-phase pyranose-to-furanose isomerization in protonated peptidoglycans" @default.
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- W3204823545 doi "https://doi.org/10.1039/d1cp03842g" @default.
- W3204823545 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34632474" @default.
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