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• W3204830905 abstract "Zeolite-templated carbon (ZTC) with a regular arrangement of single-walled sp2 carbon layers exhibits desirable materials properties such as high electrical conductivity, and have broad applications including electrochemical and charge storage. Here, we have investigated the effect of doping of nitrogen (N) and sulfur (S) on ZTC. N-doped zeolite-templated carbon (N-ZTC) with various structures, including pyridinic N, pyrrolic N, and graphitic N, has a different composition ratio depending on the temperature at which it was synthesized. The composition, electrical conductivity, and work functions of doped ZTC were investigated with X-Ray photoelectron spectroscopy (XPS), conductive atomic force microscopy (C-AFM), and Kelvin probe force microscopy (KPFM), respectively. We found that N-doped ZTC synthesized at the highest temperature (700 ℃) showed the highest graphitic N ratio and electrical conductivity, indicating an optimized N-doping effect. We show that the structure of graphitic N showed an n-type doping effect in ZTC, while pyridinic N showed a p-type doping effect. This phenomenon was explained by measuring the work function of KPFM. These results suggest a direct relationship between electrical conductivity and carbon-dopant bonding in doped microporous structures, suggesting the possibility of tuning material properties with atomic doping." @default.
• W3204830905 created "2021-10-11" @default.
• W3204830905 creator A5041659236 @default.
• W3204830905 date "2021-01-01" @default.
• W3204830905 modified "2023-10-16" @default.
• W3204830905 title "Doping Effect of Zeolite-Templated Carbon on Electrical Conductivity and Work Function" @default.
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• W3204830905 doi "https://doi.org/10.2139/ssrn.3937103" @default.
• W3204830905 hasPublicationYear "2021" @default.
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