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• W3205065441 abstract "Hydrogen bonds are arguably the most important of noncovalent interactions. The physical properties of water and the information storage in DNA depend on H-bonding, for instance. To this day, the balance between the Coulombic and covalent contributions to H-bonds is still under debate. Here, we show that H-bonded host-guest systems associate in ionic liquids, pure salts with melting point below room temperature, in which dipole-dipole electrostatic interactions should be negligible in comparison with dipole-charge interactions. Binding constants (<i>K</i>_a) obtained from titrations of four H-bonded host-guest systems in two organic solvents and two ionic liquids yield smaller yet comparable <i>K</i>_avalues in ionic liquids than in organic solvents. We also detect the association event using force spectroscopy. Our results indicate that strong H-bonds are only moderately affected by surroundings composed entirely of charges, suggesting that the balance of Coulombic to covalent forces is not tipped towards the former." @default.
• W3205065441 created "2021-10-25" @default.
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• W3205065441 date "2019-06-05" @default.
• W3205065441 modified "2023-10-14" @default.
• W3205065441 title "Strong Hydrogen Bonds Are Not Shielded in Ionic Liquids" @default.
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• W3205065441 doi "https://doi.org/10.26434/chemrxiv.8208545.v1" @default.
• W3205065441 hasPublicationYear "2019" @default.
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