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- W32052561 abstract "Layer-type transition metal dichalcogenides have proven to be very helpful model systems for the investigation of several fundamental aspects of photoelectrochemical mechanisms: the effect of crystalline asymmetry on photoelectrochemical reactivity and quantum energy conversion; the difference, in reactivity, of holes reacting via transition metal d-states and chalcogenide p-states respectively; the interfacial effect of high and low densities of surface states on photoelectrochemical mechanisms and catalysis of multielectron transfer processes. A comparative analysis of the principles involved is made with interfaces of non-layered transition metal dichalcogenides, which entirely consist of chemically reactive surface states produced by transition metal centers, d-states, which are also recognized in scanning tunnelling microscope pictures, can, provided a molecular interaction with redox species is possible, give rise to interfacial coordination chemical mechanisms, which are more efficient for electron transfer than tunnelling processes. This explains some of the materials most outstanding properties but also their limitations for solar energy conversion." @default.
- W32052561 created "2016-06-24" @default.
- W32052561 creator A5073942054 @default.
- W32052561 date "1992-01-01" @default.
- W32052561 modified "2023-09-26" @default.
- W32052561 title "Electronic Structure, Coordination Photoelectrochemical Pathways and Quantum Energy Conversion by Layered Transition Metal Dichalcogenides" @default.
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- W32052561 doi "https://doi.org/10.1007/978-94-015-1301-2_2" @default.
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