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- W3205662262 abstract "An electro-optic modulator offers the function of modulating the propagation of light in a material with electric field and enables seamless connection between electronics-based computing and photonics-based communication. The search for materials with large electro-optic coefficients and low optical loss is critical to increase the efficiency and minimize the size of electro-optic devices. We present a semi-empirical method to compute the electro-optic coefficients of ferroelectric materials by combining first-principles density-functional theory calculations with Landau-Devonshire phenomenological modeling. We apply the method to study the electro-optic constants, also called Pockels coefficients, of three paradigmatic ferroelectric oxides: BaTiO3, LiNbO3, and LiTaO3. We present their temperature-, frequency- and strain-dependent electro-optic tensors calculated using our method. The predicted electro-optic constants agree with the experimental results, where available, and provide benchmarks for experimental verification." @default.
- W3205662262 created "2021-10-25" @default.
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- W3205662262 date "2022-04-25" @default.
- W3205662262 modified "2023-09-23" @default.
- W3205662262 title "Modeling temperature, frequency, and strain effects on the linear electro-optic coefficients of ferroelectric oxides" @default.
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- W3205662262 doi "https://doi.org/10.1063/5.0090072" @default.
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