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- W3205774993 abstract "Biohydrogen production by Aqueous-Phase Reforming (APR) of glycerol was studied over nickel aluminate spinel-derived catalysts modified by Ce or Mg. As reference, an alumina supported nickel catalyst was also investigated. Catalysts were characterised by a sort of techniques in order to elucidate any structure-activity relationship, and tested for the WGS and CO hydrogenation reactions. It was concluded that the spinel catalyst allowed a better dispersion of the metallic Ni, and led to a more APR active and more hydrogen-selective catalyst. Mg and Ce doping further increased the nickel dispersion and increased basicity what could be related to their higher WGS relative reaction rate. Also, Mg doping hindered nickel reduction due to Ni-Mg interactions. Both promoters improved the stability of the textural properties under APR conditions, minimizing the formation of boehmite. Leaching of Ni was found, at lesser extent after Mg doping." @default.
- W3205774993 created "2021-10-25" @default.
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- W3205774993 date "2021-12-01" @default.
- W3205774993 modified "2023-10-16" @default.
- W3205774993 title "Biohydrogen production by glycerol Aqueous-Phase Reforming: Effect of promoters (Ce or Mg) in the NiAl2O4 spinel-derived catalysts" @default.
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- W3205774993 doi "https://doi.org/10.1016/j.jece.2021.106433" @default.
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