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• W3205988377 abstract "Natural molybdenite, an inexpensive and naturally abundant material, can be directly used as an anode material for lithium-ion batteries. However, how to release the intrinsic capacity of natural molybdenite to achieve high rate performance and high capacity is still a challenge. Herein, we introduce an innovative, effective, and one-step approach to preparing a type of heterostructure material containing 1T@2H MoS2 crafted from insertion and expansion of natural molybdenite. The metallic 1T phase formed in situ can significantly improve the electronic conductivity of MoS2. At the same time, 1T@2H MoS2 heterostructures can provide an internal electric field (E-field) to accelerate the migration rate of electrons and ions, promote the charge transfer behaviour, and ensure the reaction reversibility and lithium storage kinetics. Such worm-like 1T@2H MoS2 heterostructures also have a large specific surface area and a large number of defects, which will help shorten the lithium-ion transmission distance and provide more ion transmission channels. As a result, it exhibits a discharge capacity of 788 mA h g-1 remarkably at 100 mA g-1 after 485 cycles and stable cycling performance. It also shows excellent magnification performance of 727 mA h g-1 at 1 A g-1, compared to molybdenite concentrate. Briefly, this work's heterostructure architectures open up a new avenue for applying natural molybdenite in lithium-ion batteries, which has the potential to achieve large-scale commercial applications." @default.
• W3205988377 created "2021-10-25" @default.
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• W3205988377 date "2021-01-01" @default.
• W3205988377 modified "2023-10-18" @default.
• W3205988377 title "Construction of 1T@2H MoS₂ heterostructures <i>in situ</i> from natural molybdenite with enhanced electrochemical performance for lithium-ion batteries" @default.
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• W3205988377 doi "https://doi.org/10.1039/d1ra05565h" @default.
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