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- W3206094966 abstract "Recently it was shown that the MnIII(TPPS) – hydrogen peroxide system in alkaline media exhibits a vigorous catalase activity. Intermediate (TPPS)MnVO formed in a catalytic cycle in the system is an efficient degrading agent for a model dye, Orange II, in carbonate buffers. The high efficacy of the catalyst under these conditions is attributed to the generation of strongly oxidising percarbonate ions, a commonly known effect. The detailed study on the MnIII(TPPS) catalysed rapid degradation of methylene blue by hydrogen peroxide, performed using stopped-flow electronic spectroscopy as a function of the catalyst, hydrogen peroxide, pH and carbonate concentrations reported herein, has surprisingly evidenced a minor role of percarbonate in the overall catalytic cycle." @default.
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- W3206094966 date "2021-12-01" @default.
- W3206094966 modified "2023-10-16" @default.
- W3206094966 title "Mechanistic details of the catalytic degradation of methylene blue by hydrogen peroxide in basic solution. The unexpected innocence of percarbonate" @default.
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- W3206094966 doi "https://doi.org/10.1016/j.poly.2021.115507" @default.
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