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• W3206188840 abstract "Two new chemically stable metalloporphyrin-bridged metal-catechol frameworks, InTCP-Co and FeTCP-Co, were constructed to achieve artificial photosynthesis without additional sacrificial agents and photosensitizers. The CO2 photoreduction rate over FeTCP-Co considerably exceeds that obtained over InTCP-Co, and the incorporation of uncoordinated hydroxyl groups, associated with catechol, into the network further promotes the photocatalytic activity. The iron-oxo coordination chain assists energy band alignment and provides a redox-active site, and the uncoordinated hydroxyl group contributes to the visible-light absorptance, charge-carrier transfer, and CO2 -scaffold affinity. With a formic acid selectivity of 97.8 %, FeTCP-OH-Co affords CO2 photoconversion with a reaction rate 4.3 and 15.7 times higher than those of FeTCP- Co and InTCP-Co, respectively. These findings are also consistent with the spectroscopic study and DFT calculation." @default.
• W3206188840 created "2021-10-25" @default.
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• W3206188840 date "2021-11-25" @default.
• W3206188840 modified "2023-10-03" @default.
• W3206188840 title "Energy Band Alignment and Redox‐Active Sites in Metalloporphyrin‐Spaced Metal‐Catechol Frameworks for Enhanced CO₂ Photoreduction" @default.
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• W3206188840 doi "https://doi.org/10.1002/anie.202111622" @default.
• W3206188840 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34652055" @default.
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