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- W3206417765 abstract "Quantitative characterization of the energy dissipative zone around the crack tip is the central issue in fracture mechanics of soft materials. In this research, we present a mechanochemical technique to visualize the bond scission of the first network in the damage zone of tough double-network hydrogels. The mechanoradicals generated by polymer chain scission are employed to initiate polymerization of a thermoresponsive polymer, which is visualized by a fluorophore. This technique records the spatial distribution of internal fracturing from the fractured surface to the bulk, which provides the spatial profiles of stress, strain, and energy dissipation around the crack-tip. The characterized results suggest that, in addition to the dissipation in relatively narrow yielded zone which is mostly focused in the previous works, the dissipation in wide pre-yielding zone and the intrinsic fracture energy have also significant contribution to the fracture energy of a DN gel." @default.
- W3206417765 created "2021-10-25" @default.
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- W3206417765 date "2020-06-26" @default.
- W3206417765 modified "2023-10-16" @default.
- W3206417765 title "Crack Tip Field of a Double-Network Gel: Visualizing Covalent Bond Scission by Mechanoradical Polymerization" @default.
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- W3206417765 doi "https://doi.org/10.26434/chemrxiv.12555419.v1" @default.
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