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• W3206699504 startingPage "5816" @default.
• W3206699504 abstract "Electrocatalytic CO$_2$RR is an interfacial process, involving a minimum of three phases at the contact point of gaseous CO$_2$ with the electrodic surface and the liquid electrolyte. As a consequence, surface chemistry at composite interfaces plays a central role for CO$_2$RR selectivity and catalysis. Each interface defines a functional boundary, where active sites are exposed to a unique environment with respect to distal sites in the bulk or organic and inorganic materials. While the individual role of each component-type is hardly predictable a-solo, the interface ensemble works via a strategic interplay of individual effects, including: (i) enhanced electrical conductivity, (ii) high surface area and exposure of the interfacial catalytic sites, (iii) favorable transport and feeding of reactants, (iv) complementary interactions for the on/off stabilization of cascade intermediates, (v) a secondary sphere assistance to lower the activation energy of bottleneck steps, (vi) a reinforced robustness and long-term operation stability by mutual protection and/or healing mechanisms. Selected CO$_2$RR case studies are compared and contrasted to highlight how the organic domains of carbon nanostructures merge with metal and metal-oxide active sites to separate tasks but also to turn them into a cooperative asset of mutual interactions, thus going beyond the classic Divide et Impera rule." @default.
• W3206699504 created "2021-10-25" @default.
• W3206699504 creator A5008190147 @default.
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• W3206699504 creator A5074191348 @default.
• W3206699504 date "2021-01-01" @default.
• W3206699504 modified "2023-10-17" @default.
• W3206699504 title "Electrocatalytic CO₂ reduction: role of the cross-talk at nano-carbon interfaces" @default.
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