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• W3206777410 endingPage "132857" @default.
• W3206777410 startingPage "132857" @default.
• W3206777410 abstract "• Inactive g-C 3 N 4 was functionalized to be highly efficient Hg 0 adsorbents. • In 2 S 3 /g-C 3 N 4 exhibits excellent Hg 0 adsorption performance in a wide temperature range of 80 to 240 °C. • In 2 S 3 /g-C 3 N 4 performs an excellent adsorption capacity (14.78 mg/g). • In 2 S 3 /g-C 3 N 4 converts the adsorbed mercury into stable HgS. Mercury emission from coal-fired power plants has posed a great threat to the environment and human, and reducing and controlling mercury emissions has become a global environmental issue. In this work, the In 2 S 3 /g-C 3 N 4 adsorbent was prepared by simple hydrothermal method to achieve efficient removal of Hg 0 from coal-fired flue gas. When the loading value of In 2 S 3 was 40 %, the effect of removing Hg 0 by as-synthesized IC-40 was the best. IC-40 showed excellent Hg 0 adsorption performance in a temperature range of 80–240 °C. Under the condition of 120 °C and N 2 atmosphere, the Hg 0 adsorption capacity of the synthesized IC-40 reached 14.78 mg/g. The study on the impacts of flue gas components demonstrate that IC-40 has good resistance to nitric oxide, and has a slight inhibitory effect by SO 2 and water vapor. According to the results of XPS and Hg-TPD, the formed main mercury compound is extremely stable HgS. In addition, DFT was conducted to calculate the adsorption energy of Hg 0 on In 2 S 3 (1 1 0) surface, which further illustrated the sulfur site served as stable adsorption site to convert Hg 0 into HgS. From the above analysis, IC-40 as an efficient and scientific adsorbent to remove Hg 0 from coal-fired power plants is a promising technical method." @default.
• W3206777410 created "2021-10-25" @default.
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• W3206777410 date "2022-02-01" @default.
• W3206777410 modified "2023-09-30" @default.
• W3206777410 title "Spherical In2S3 anchored on g-C3N4 nanosheets for efficient elemental mercury removal in the wide temperature range" @default.
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• W3206777410 doi "https://doi.org/10.1016/j.cej.2021.132857" @default.
• W3206777410 hasPublicationYear "2022" @default.
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