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• W3206834757 abstract "CO2 emissions can be transformed into high-added-value commodities through CO2 electrocatalysis; however, efficient low-cost electrocatalysts are needed for global scale-up. Inspired by other emerging technologies, the authors report the development of a gas diffusion electrode containing highly dispersed Ag sites in a low-cost Zn matrix. This catalyst shows unprecedented Ag mass activity for CO production: -614 mA cm-2 at 0.17 mg of Ag. Subsequent electrolyte engineering demonstrates that halide anions can further improve stability and activity of the Zn-Ag catalyst, outperforming pure Ag and Au. Membrane electrode assemblies are constructed and coupled to a microbial process that converts the CO to acetate and ethanol. Combined, these concepts present pathways to design catalysts and systems for CO2 conversion toward sought-after products." @default.
• W3206834757 created "2021-10-25" @default.
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• W3206834757 date "2021-10-21" @default.
• W3206834757 modified "2023-10-14" @default.
• W3206834757 title "Designing a Zn–Ag Catalyst Matrix and Electrolyzer System for CO ₂ Conversion to CO and Beyond" @default.
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• W3206834757 doi "https://doi.org/10.1002/adma.202103963" @default.
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