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- W3206858081 abstract "Two rare earth coordination polymers named {[La6(C9H11N2O4)11(H2O)2(OH)2]⋅Br5}n (1) and [Gd(C9H11N2O4)(C2O4)(H2O)]n (2) (C9H11N2O42‒ = 1,3-bis(1-carboxylatoethyl) imidazolium ion, C2O42- = oxalate) were solvothermally synthesized using zwitterionic 1,3-bis(1-carboxylatoethyl)imidazolium bromide as ligand. 1 and 2 were both structurally characterized by single crystal X-ray diffraction, and their thermodynamic properties and magnetic properties of 2 were studied. In the 3D structure of 1, La3+ ions are all ten-coordinated and exhibit three different coordination environments. This 3D structure of 1 is formed by La−O coordination bonds with Br− located in the cavities through H-bond and electrostatic attraction. Different from 1, all Gd3+ ions in 2 have the same eight-coordinated environment. These two coordination polymers both have good thermostability until 323 °C for 1 and 375 °C for 2, and then decompose giving rise to La2O3 and Gd2O3, respectively. The magnetic behaviors of 2 are measured in the temperature range 2–300 K." @default.
- W3206858081 created "2021-10-25" @default.
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- W3206858081 date "2022-02-01" @default.
- W3206858081 modified "2023-10-13" @default.
- W3206858081 title "Two Novel Rare Earth Coordination Polymers Derived from Zwitterionic 1,3-Bis(1-carboxylatoethyl)imidazolium Bromide: Structures and Magnetic Properties" @default.
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- W3206858081 doi "https://doi.org/10.1016/j.molstruc.2021.131665" @default.
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