Matches in SemOpenAlex for { <https://semopenalex.org/work/W3207109660> ?p ?o ?g. }
- W3207109660 abstract "Adsorbed atoms (adatoms) coupled to the matrix of solid state host materials as impurities can significantly modify their properties. Especially in low-dimensional materials, such as one-dimensional organic polymer chains or quasi-one-dimensional graphene nanoribbons, intriguing manipulation of the optical properties, such as the absorption cross section, is possible. The most widely used approach to couple quantum emitters to optical antennas is based on the Purcell effect. This formalism, however, does not comprise charge transfer from the emitter to the antenna, but only spontaneous emission of the quantum emitter into the tailored photonic environment, that is evoked by the antenna. To capture such effects, we present a tight-binding formalism to couple an adatom to a finite Su-Schrieffer-Heeger chain, where the former is treated as a two-level system and the latter acts as an optical antenna. We systematically analyze how the coupling strength and the position of the adatom influence the optical properties of the molecular chains in the model. We take into account charge transfer from the adatom to the antenna and vice versa via an inter-system hopping parameter, and also include Coulomb interaction within the antenna as well as between the adatom and the antenna. We show that coupling the adatom to one of the bulk atoms of the linear chain results in a substantial change in optical properties already for comparatively small coupling strengths. We also find that the position of the adatom crucially determines if and how the optical properties of the chains are altered. Therefore, we identify this adatom-chain hybrid system as a tunable platform for light-matter interaction at the nanoscale." @default.
- W3207109660 created "2021-10-25" @default.
- W3207109660 creator A5032268062 @default.
- W3207109660 creator A5036281595 @default.
- W3207109660 creator A5044528120 @default.
- W3207109660 creator A5054748851 @default.
- W3207109660 creator A5060759834 @default.
- W3207109660 creator A5076705483 @default.
- W3207109660 creator A5082661877 @default.
- W3207109660 date "2021-12-13" @default.
- W3207109660 modified "2023-10-18" @default.
- W3207109660 title "Modification of the optical properties of molecular chains upon coupling to adatoms" @default.
- W3207109660 cites W1793289399 @default.
- W3207109660 cites W1809201061 @default.
- W3207109660 cites W1969192068 @default.
- W3207109660 cites W1971472669 @default.
- W3207109660 cites W1974447177 @default.
- W3207109660 cites W1976157202 @default.
- W3207109660 cites W1977955686 @default.
- W3207109660 cites W1978245542 @default.
- W3207109660 cites W1978392299 @default.
- W3207109660 cites W1978762857 @default.
- W3207109660 cites W1979720427 @default.
- W3207109660 cites W1981103785 @default.
- W3207109660 cites W1982840202 @default.
- W3207109660 cites W1983136922 @default.
- W3207109660 cites W1986394157 @default.
- W3207109660 cites W1987636344 @default.
- W3207109660 cites W1992040324 @default.
- W3207109660 cites W1992148234 @default.
- W3207109660 cites W1994424786 @default.
- W3207109660 cites W1996826343 @default.
- W3207109660 cites W2002649952 @default.
- W3207109660 cites W2009742332 @default.
- W3207109660 cites W2009759993 @default.
- W3207109660 cites W2012738884 @default.
- W3207109660 cites W2017777166 @default.
- W3207109660 cites W2026362106 @default.
- W3207109660 cites W2033808935 @default.
- W3207109660 cites W2036537498 @default.
- W3207109660 cites W2043603313 @default.
- W3207109660 cites W2043638708 @default.
- W3207109660 cites W2048119540 @default.
- W3207109660 cites W2050315976 @default.
- W3207109660 cites W2050392107 @default.
- W3207109660 cites W2056766189 @default.
- W3207109660 cites W2059633429 @default.
- W3207109660 cites W2072458642 @default.
- W3207109660 cites W2072703702 @default.
- W3207109660 cites W2075978951 @default.
- W3207109660 cites W2076757970 @default.
- W3207109660 cites W2077018894 @default.
- W3207109660 cites W2082197329 @default.
- W3207109660 cites W2085155410 @default.
- W3207109660 cites W2089843538 @default.
- W3207109660 cites W2094171888 @default.
- W3207109660 cites W2110051306 @default.
- W3207109660 cites W2124737612 @default.
- W3207109660 cites W2133622178 @default.
- W3207109660 cites W2141240101 @default.
- W3207109660 cites W2149816900 @default.
- W3207109660 cites W2166812142 @default.
- W3207109660 cites W2319394938 @default.
- W3207109660 cites W2336764616 @default.
- W3207109660 cites W2464969954 @default.
- W3207109660 cites W2515293542 @default.
- W3207109660 cites W2528145116 @default.
- W3207109660 cites W2554178941 @default.
- W3207109660 cites W2742072372 @default.
- W3207109660 cites W2754319903 @default.
- W3207109660 cites W2763461985 @default.
- W3207109660 cites W2776174376 @default.
- W3207109660 cites W2804955439 @default.
- W3207109660 cites W2901024572 @default.
- W3207109660 cites W2971404577 @default.
- W3207109660 cites W2980696205 @default.
- W3207109660 cites W3036100162 @default.
- W3207109660 cites W3085741731 @default.
- W3207109660 cites W3097806387 @default.
- W3207109660 cites W3097978959 @default.
- W3207109660 cites W3102897980 @default.
- W3207109660 cites W3103013820 @default.
- W3207109660 cites W3103879548 @default.
- W3207109660 cites W3104001197 @default.
- W3207109660 cites W3105266520 @default.
- W3207109660 cites W3135537862 @default.
- W3207109660 doi "https://doi.org/10.1103/physrevb.104.235414" @default.
- W3207109660 hasPublicationYear "2021" @default.
- W3207109660 type Work @default.
- W3207109660 sameAs 3207109660 @default.
- W3207109660 citedByCount "2" @default.
- W3207109660 countsByYear W32071096602022 @default.
- W3207109660 crossrefType "journal-article" @default.
- W3207109660 hasAuthorship W3207109660A5032268062 @default.
- W3207109660 hasAuthorship W3207109660A5036281595 @default.
- W3207109660 hasAuthorship W3207109660A5044528120 @default.
- W3207109660 hasAuthorship W3207109660A5054748851 @default.
- W3207109660 hasAuthorship W3207109660A5060759834 @default.
- W3207109660 hasAuthorship W3207109660A5076705483 @default.
- W3207109660 hasAuthorship W3207109660A5082661877 @default.