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- W3207301637 abstract "The origin of the coil-globule transition for water-soluble thermoresponsive polymers frequently used in nanomaterials remains elusive. Using polypropylene oxide as an example we demonstrate by means of atomistic molecular dynamics simulations that temperature-induced increase in the sequence length of monomers that are not hydrogen bonded to water drives the coil-globule transition. Longer chains statistically exhibit longer sequences which serve as nucleation sites for hydrophobic cluster formation, facilitating chain collapse at lower temperature in agreement with experimental data." @default.
- W3207301637 created "2021-10-25" @default.
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- W3207301637 date "2021-10-12" @default.
- W3207301637 modified "2023-10-14" @default.
- W3207301637 title "Hydrogen Bonding Sequence Directed Coil-Globule Transition in Water Soluble Thermoresponsive Polymers" @default.
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- W3207301637 doi "https://doi.org/10.1103/physrevlett.127.167801" @default.
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