Matches in SemOpenAlex for { <https://semopenalex.org/work/W3207575287> ?p ?o ?g. }
- W3207575287 endingPage "819" @default.
- W3207575287 startingPage "812" @default.
- W3207575287 abstract "The design of efficient and robust non-precious metal electrocatalysts towards oxygen evolution reaction (OER) is of great value for developing green energy technologies. The in-situ formed high-valence (oxy)hydroxides species during the reconstruction process of pre-catalysts are recognized as the real contributing sites for OER. However, pre-catalysts generally undergo a slow and inadequate self-reconstruction. Herein, we reported a PO43− optimized CoFe-based OER catalysts with amorphous structure, which enables a fast and deep reconstruction during the OER process. The amorphous structure induced by ligands PO43− is prone to evolution and further form active species for OER. The electron interaction between metal sites can be modulated by electron-rich PO43−, which promotes generation of high active CoOOH. Simultaneously, the etching of PO43− from the pre-catalysts during the catalytic process is in favor of accelerating the self-reconstruction. As a result, as-prepared pre-catalyst can generate high active CoOOH at a low potential of 1.4 V and achieve an in-depth reconstructed nanosheet structure with abundant OER active sites. Our work provides a promising design of pre-catalysts for realizing efficient catalysis of water oxidation." @default.
- W3207575287 created "2021-10-25" @default.
- W3207575287 creator A5058986413 @default.
- W3207575287 creator A5059651484 @default.
- W3207575287 creator A5086063023 @default.
- W3207575287 date "2023-06-01" @default.
- W3207575287 modified "2023-10-14" @default.
- W3207575287 title "A fast and in-depth self-reconstruction of anion ligands optimized CoFe-based pre-catalysts for water oxidation" @default.
- W3207575287 cites W2058267335 @default.
- W3207575287 cites W2137776484 @default.
- W3207575287 cites W2151019712 @default.
- W3207575287 cites W2165291607 @default.
- W3207575287 cites W2315225874 @default.
- W3207575287 cites W2326257739 @default.
- W3207575287 cites W2332386396 @default.
- W3207575287 cites W2552909336 @default.
- W3207575287 cites W2557308056 @default.
- W3207575287 cites W2743195422 @default.
- W3207575287 cites W2751087297 @default.
- W3207575287 cites W2790704802 @default.
- W3207575287 cites W2801806667 @default.
- W3207575287 cites W2885447879 @default.
- W3207575287 cites W2896114205 @default.
- W3207575287 cites W2899283893 @default.
- W3207575287 cites W2899400793 @default.
- W3207575287 cites W2901644505 @default.
- W3207575287 cites W2904657824 @default.
- W3207575287 cites W2909774500 @default.
- W3207575287 cites W2910857126 @default.
- W3207575287 cites W2915123062 @default.
- W3207575287 cites W2941438073 @default.
- W3207575287 cites W2955003935 @default.
- W3207575287 cites W2955643367 @default.
- W3207575287 cites W2962944603 @default.
- W3207575287 cites W2967299079 @default.
- W3207575287 cites W2968364898 @default.
- W3207575287 cites W2977238283 @default.
- W3207575287 cites W2979773918 @default.
- W3207575287 cites W2999930969 @default.
- W3207575287 cites W3012557858 @default.
- W3207575287 cites W3034716826 @default.
- W3207575287 cites W3035082486 @default.
- W3207575287 cites W3044292408 @default.
- W3207575287 cites W3092550585 @default.
- W3207575287 cites W3105173746 @default.
- W3207575287 cites W3108609492 @default.
- W3207575287 cites W3120721923 @default.
- W3207575287 cites W3123345378 @default.
- W3207575287 cites W3126294363 @default.
- W3207575287 cites W3126971546 @default.
- W3207575287 cites W3140549205 @default.
- W3207575287 cites W3143081366 @default.
- W3207575287 cites W3159160367 @default.
- W3207575287 doi "https://doi.org/10.1016/j.gee.2021.10.002" @default.
- W3207575287 hasPublicationYear "2023" @default.
- W3207575287 type Work @default.
- W3207575287 sameAs 3207575287 @default.
- W3207575287 citedByCount "2" @default.
- W3207575287 countsByYear W32075752872022 @default.
- W3207575287 countsByYear W32075752872023 @default.
- W3207575287 crossrefType "journal-article" @default.
- W3207575287 hasAuthorship W3207575287A5058986413 @default.
- W3207575287 hasAuthorship W3207575287A5059651484 @default.
- W3207575287 hasAuthorship W3207575287A5086063023 @default.
- W3207575287 hasBestOaLocation W32075752871 @default.
- W3207575287 hasConcept C127413603 @default.
- W3207575287 hasConcept C135473242 @default.
- W3207575287 hasConcept C147789679 @default.
- W3207575287 hasConcept C161790260 @default.
- W3207575287 hasConcept C168900304 @default.
- W3207575287 hasConcept C171250308 @default.
- W3207575287 hasConcept C17525397 @default.
- W3207575287 hasConcept C178790620 @default.
- W3207575287 hasConcept C179104552 @default.
- W3207575287 hasConcept C185592680 @default.
- W3207575287 hasConcept C192562407 @default.
- W3207575287 hasConcept C35590869 @default.
- W3207575287 hasConcept C42360764 @default.
- W3207575287 hasConcept C51967427 @default.
- W3207575287 hasConcept C52859227 @default.
- W3207575287 hasConcept C56052488 @default.
- W3207575287 hasConcept C65165184 @default.
- W3207575287 hasConceptScore W3207575287C127413603 @default.
- W3207575287 hasConceptScore W3207575287C135473242 @default.
- W3207575287 hasConceptScore W3207575287C147789679 @default.
- W3207575287 hasConceptScore W3207575287C161790260 @default.
- W3207575287 hasConceptScore W3207575287C168900304 @default.
- W3207575287 hasConceptScore W3207575287C171250308 @default.
- W3207575287 hasConceptScore W3207575287C17525397 @default.
- W3207575287 hasConceptScore W3207575287C178790620 @default.
- W3207575287 hasConceptScore W3207575287C179104552 @default.
- W3207575287 hasConceptScore W3207575287C185592680 @default.
- W3207575287 hasConceptScore W3207575287C192562407 @default.
- W3207575287 hasConceptScore W3207575287C35590869 @default.
- W3207575287 hasConceptScore W3207575287C42360764 @default.
- W3207575287 hasConceptScore W3207575287C51967427 @default.
- W3207575287 hasConceptScore W3207575287C52859227 @default.
- W3207575287 hasConceptScore W3207575287C56052488 @default.