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• W3207772091 abstract "Electrode (including cathode and anode) /electrolyte interfaces play a vital role in determining battery performance. Especially, high-voltage lithium metal batteries (HVLMBs) with the Ni-rich layered oxide ternary cathode (NCM) can be considered a promising energy storage technology due to their outstanding energy density. However, it is still extremely challenging to address the unstable electrode/electrolyte interface and structural collapse of polycrystalline NCM at high voltage, greatly restraining its practical applications. In this work, a novel electrolyte additive, tris(2-cyanoethyl) borate (TCEB), has been used to construct the robust nitrogen (N) and boron (B)-rich protective films on single-crystal LiNi0.6Co0.1Mn0.3O2 (SNCM) cathode and lithium metal anode surfaces, which could effectively mitigate parasitic reactions against electrolyte corrosion and retain the structural integrity of electrode. Remarkably, the SNCM||Li metal cell using TCEB-containing electrolyte maintains unprecedentedly superb capacity retention of 80% after 100 cycles at an ultrahigh charging voltage of 4.7 V (versus Li/Li+). This finding provides a valuable reference to construct a stable electrode/electrolyte interface for the HVLMBs with achieving high-energy density." @default.
• W3207772091 created "2021-10-25" @default.
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• W3207772091 date "2022-02-01" @default.
• W3207772091 modified "2023-10-15" @default.
• W3207772091 title "Improving interfacial stability of ultrahigh-voltage lithium metal batteries with single-crystal Ni-rich cathode via a multifunctional additive strategy" @default.
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• W3207772091 doi "https://doi.org/10.1016/j.jcis.2021.10.061" @default.
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• W3207772091 hasPublicationYear "2022" @default.
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