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- W3207798517 abstract "Spontaneous emission of quantum emitters can be enhanced by increasing the local density of optical states, whereas engineering dipole-dipole interactions requires modifying the two-point spectral density function. Here, we experimentally demonstrate long-range dipole-dipole interactions (DDIs) mediated by surface lattice resonances in a plasmonic nanoparticle lattice. Using angle-resolved spectral measurements and fluorescence lifetime studies, we show that unique nanophotonic modes mediate long-range DDI between donor and acceptor molecules. We observe significant and persistent DDI strengths for a range of densities that map to ∼800 nm mean nearest-neighbor separation distance between donor and acceptor dipoles, a factor of ∼100 larger than free space. Our results pave the way to engineer and control long-range DDIs between an ensemble of emitters at room temperature." @default.
- W3207798517 created "2021-10-25" @default.
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- W3207798517 date "2021-10-21" @default.
- W3207798517 modified "2023-10-12" @default.
- W3207798517 title "Long-Range Dipole–Dipole Interactions in a Plasmonic Lattice" @default.
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- W3207798517 doi "https://doi.org/10.1021/acs.nanolett.1c02835" @default.
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- W3207798517 hasPublicationYear "2021" @default.
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