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• W3207808889 endingPage "1496" @default.
• W3207808889 startingPage "1489" @default.
• W3207808889 abstract "Electrocatalytic N2 reduction reaction (NRR) provides a promising route for NH3 production under ambient conditions to replace traditional Haber-Bosch process. For this purpose, efficient NRR electrocatalysts with high NH3 yield rate and high Faradaic efficiency (FE) are required. Cu-based materials have been recognized catalytic active for some multi-electron-involved reduction reactions and usually exhibit inferior catalytic activities for hydrogen evolution reaction. We report here the preparation and characterization of a series of Cu-based nanowires array (NA) catalysts in situ grown on Cu foam (CF) substrate, including Cu(OH)2 NA/CF, Cu3N NA/CF, Cu3P NA/CF, CuO NA/CF and Cu NA/CF, which are directly used as self-supported catalytic electrodes for NRR. The electrochemical results show that CuO NA/CF achieves a highest NH3 yield rate of 1.84 × 10-9 mol s-1 cm-2, whereas Cu NA/CF possesses a highest FE of 18.2% for NH3 production at -0.1 V versus reversible hydrogen electrode in 0.1 M Na2SO4. Such catalytic performances are superior to most of recently reported metal-based NRR electrocatalysts. The contact angle measurements and the simulated calculations are carried out to reveal the important role of the superaerophobic NA surface structure for efficient NRR electrocatalysis." @default.
• W3207808889 created "2021-10-25" @default.
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• W3207808889 date "2022-02-01" @default.
• W3207808889 modified "2023-10-06" @default.
• W3207808889 title "Superaerophobic copper-based nanowires array for efficient nitrogen reduction" @default.
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• W3207808889 doi "https://doi.org/10.1016/j.jcis.2021.10.062" @default.
• W3207808889 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34742068" @default.
• W3207808889 hasPublicationYear "2022" @default.
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