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- W3207816590 abstract "A theoretical approach is developed for the Herman-Wallis factors describing the variation of the line intensities caused by rovibrational interaction in a linear molecule. In the case of ${ensuremath{nu}}_{2}$ and ${ensuremath{nu}}_{3}$ fundamentals and the ${ensuremath{nu}}_{1}+{ensuremath{nu}}_{3}/2{ensuremath{nu}}_{2}+{ensuremath{nu}}_{3}$ resonance combination band in a ${mathrm{CO}}_{2}$ molecule, our theory is capable of generating reliable numerical estimates for the linear Herman-Wallis coefficients without recourse to complicated algebra. On the assumption of nearly free rotating monomers, an analog of the Herman-Wallis factors is introduced for the dipole-forbidden ${ensuremath{nu}}_{2}+{ensuremath{nu}}_{3}$ band, which manifests itself in ${mathrm{CO}}_{2}$ collision-induced absorption (CIA). The rovibrational perturbation is appropriate to explain a pronounced crossflow of intensity among rovibrational branches in a virtually rotationally unresolved CIA envelope." @default.
- W3207816590 created "2021-10-25" @default.
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- W3207816590 date "2021-10-11" @default.
- W3207816590 modified "2023-10-12" @default.
- W3207816590 title "Theory of rovibrational line intensities in allowed and collision-induced absorption spectra of linear molecules" @default.
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- W3207816590 doi "https://doi.org/10.1103/physreva.104.042805" @default.
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