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• W3207831249 endingPage "16438" @default.
• W3207831249 startingPage "16429" @default.
• W3207831249 abstract "The rare combination of InIII 5p and ZnII 3d in the presence of a structure-oriented TDP6- ligand led to a robust hybrid material of {(Me2NH2)[InZn(TDP)(OH2)]·4DMF·4H2O}n (NUC-42) with the interlaced hierarchical nanochannels (hexagonal and cylindrical) shaped by six rows of undocumented [InZn(CO2)6(OH2)] clusters, which represented the first 5p-3d nanochannel-based heterometallic metal-organic framework. With respect to the multifarious symbiotic Lewis acid-base and Brønsted acid sites in the high porous framework, the catalytic performance of activated NUC-42a upon CO2 cycloaddition with styrene oxide was evaluated under solvent-free conditions with 1 atm of CO2 pressure, which exhibited that the reaction could be well completed at ambient temperature within 48 h or at 60 °C within 4 h with high yield and selectivity. Moreover, because of the acidic function of metal sites and a central free pyridine in the TDP6- ligand, deacetalization-Knoevenagel condensation of acetals and malononitrile could be efficiently facilitated by an activated sample of NUC-42a under lukewarm conditions." @default.
• W3207831249 created "2021-10-25" @default.
• W3207831249 creator A5022538052 @default.
• W3207831249 creator A5055021669 @default.
• W3207831249 creator A5055032252 @default.
• W3207831249 creator A5088133681 @default.
• W3207831249 date "2021-10-13" @default.
• W3207831249 modified "2023-10-14" @default.
• W3207831249 title "Nanochannel {InZn}–Organic Framework with a High Catalytic Performance on CO₂ Chemical Fixation and Deacetalization–Knoevenagel Condensation" @default.
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• W3207831249 doi "https://doi.org/10.1021/acs.inorgchem.1c02262" @default.
• W3207831249 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34644055" @default.
• W3207831249 hasPublicationYear "2021" @default.
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