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- W3208018305 abstract "Development of multi-ligand metal-organic frameworks (MOFs) and derived heteroatom-doped composites as efficient non-noble metal-based catalysts is highly desirable. However, rational design of these materials with controllable composition and structure remains a challenge. In this study, novel hierarchical N-doped CuO/Cu composites were synthesized by assembling dual-ligand MOFs via a solvent-induced coordination modulation/low-temperature pyrolysis method. Different from a homogeneous system, our heterogeneous nucleation strategy provided more flexible and cost-effective MOF production and offered efficient direction/shape-controlled synthesis, resulting in a faster reaction and more complete conversion. After pyrolysis, they further transformed to a unique metal/carbon matrix with regular morphology and, as a hot template, guided the orderly generation of metal oxides, eliminating sintering and agglomeration of metal oxides and initiating a synergistic effect between the N-doped metal oxide/metal and carbon matrix. The prepared N-doped CuO/Cu catalysts held unique water resistance and superior catalytic activity (100% CO conversion at 140 °C)." @default.
- W3208018305 created "2021-11-08" @default.
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- W3208018305 date "2021-10-25" @default.
- W3208018305 modified "2023-10-13" @default.
- W3208018305 title "Hierarchical N-Doped CuO/Cu Composites Derived from Dual-Ligand Metal–Organic Frameworks as Cost-Effective Catalysts for Low-Temperature CO Oxidation" @default.
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- W3208018305 doi "https://doi.org/10.1021/acsomega.1c03877" @default.
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