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- W3208222238 abstract "Development of high-performance mixed potential gas sensors is challenging, due to a lack of understanding towards the key material properties affecting the sensing performance. Herein, with a combined theoretical-experimental study, we show that mixed potential response of perovskite oxides to hydrogen correlates to ratio of the electroactivities (exchange current densities or polarization resistances) under typical Tafel-type sensing condition. Experimental results obtained for five different perovskites indicate that a greater ratio of activities for the hydrogen oxidation reaction and the oxygen reduction one favors larger response, following a semi-logarithm relation, which agrees well with the theoretical prediction. The activity ratio could serve as a descriptor of response that is potentially applicable to different materials and target gases. These findings link mixed potential gas response to intrinsic materials properties, and would help guide the design of high response materials." @default.
- W3208222238 created "2021-11-08" @default.
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- W3208222238 date "2022-02-01" @default.
- W3208222238 modified "2023-10-14" @default.
- W3208222238 title "The relation between mixed-potential hydrogen response and electrochemical activities for perovskite oxides" @default.
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- W3208222238 doi "https://doi.org/10.1016/j.snb.2021.130988" @default.
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